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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: A. Tsekeri; A. Gialitaki; A. Gialitaki; A. Gialitaki; +55 Authors

    Abstract. The European Aerosol Research Lidar Network (EARLINET), part of the Aerosols, Clouds and Trace gases Research Infrastructure (ACTRIS), organized an intensive observational campaign in May 2020, with the objective of monitoring the atmospheric state over Europe during the COVID-19 lockdown and relaxation period. Besides the standard operational processing of the lidar data in EARLINET, for seven EARLINET sites having collocated sun-photometric observations in the Aerosol Robotic Network (AERONET), a network exercise was held in order to derive profiles of the concentration and effective column size distributions of the aerosols in the atmosphere, by applying the GRASP/GARRLiC (from Generalized Aerosol Retrieval from Radiometer and Lidar Combined data – GARRLiC – part of the Generalized Retrieval of Atmosphere and Surface Properties – GRASP) inversion algorithm. The objective of this network exercise was to explore the possibility of identifying the anthropogenic component and of monitoring its spatial and temporal characteristics in the COVID-19 lockdown and relaxation period. While the number of cases is far from being statistically significant so as to provide a conclusive description of the atmospheric aerosols over Europe during this period, this network exercise was fundamental to deriving a common methodology for applying GRASP/GARRLiC to a network of instruments with different characteristics. The limits of the approach are discussed, in particular the missing information close to the ground in the lidar measurements due to the instrument geometry and the sensitivity of the GRASP/GARRLiC retrieval to the settings used, especially for cases with low aerosol optical depth (AOD) like the ones we show here. We found that this sensitivity is well-characterized in the GRASP/GARRLiC products, since it is included in their retrieval uncertainties.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Atmospheric Measurem...arrow_drop_down
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    Atmospheric Measurement Techniques
    Article . 2023 . Peer-reviewed
    License: CC BY
    Data sources: Crossref
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    DOAJ
    Article . 2023
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Atmospheric Measurem...arrow_drop_down
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      Atmospheric Measurement Techniques
      Article . 2023 . Peer-reviewed
      License: CC BY
      Data sources: Crossref
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Rémy Ballot; Nicolas Guilpart; Marie-Hélène Jeuffroy;

    Crop diversification is considered a key element of agroecological transition, whereas current dominant cropping systems are known to rely on only a few crop species – like cereals in Europe. To assess the benefits of crop diversification at a large scale, an accurate description of current crop sequences is required as a baseline. However, such a description is lacking at the scale of Europe. Here, we developed the first map of dominant crop sequences in Europe for the period 2012–2018. We used the Land Use Cover Area frame statistical Survey (LUCAS) dataset that provides temporally incomplete (2012, 2015 and 2018) land cover information from a stable grid of points covering Europe. Eight crop sequence types were identified using hierarchical clustering implemented on LUCAS data and mapped over Europe. We show, in France, that the relative importance of these eight crop sequence types (as estimated from LUCAS data) was highly consistent with those derived from an almost spatially exhaustive temporally complete national dataset (the French Land Parcel Identification System) for the same period, thus validating the method and typology for this country. Land use (i.e. crop production area) derived from our map of dominant crop sequences was also highly consistent with land use reported by official statistics at both national and European levels, validating the approach at a European scale. This first map of dominant crop sequences in Europe should be useful for future studies dealing with agricultural issues that are sensitive to crop rotations. The map of dominant crop sequence types in Europe derived from our work is available at https://doi.org/10.5281/zenodo.7016986 (Ballot et al., 2022).

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Earth System Science...arrow_drop_down
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    Earth System Science Data (ESSD)
    Article . 2023 . Peer-reviewed
    License: CC BY
    Data sources: Crossref
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Earth System Science Data (ESSD)
    Other literature type . 2023
    DOAJ
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      Earth System Science Data (ESSD)
      Article . 2023 . Peer-reviewed
      License: CC BY
      Data sources: Crossref
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Earth System Science Data (ESSD)
      Other literature type . 2023
      DOAJ
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    Authors: Sicart, Jean Emmanuel; Ramseyer, Victor; Picard, Ghislain; Arnaud, Laurent; +15 Authors

    Forests strongly modify the accumulation, metamorphism and melting of snow in midlatitude and high-latitude regions. Recently, snow routines in hydrological and land surface models were improved to incorporate more accurate representations of forest snow processes, but model intercomparison projects have identified deficiencies, partly due to incomplete knowledge of the processes controlling snow cover in forests. The Snow Under Forest (SnoUF) project was initiated to enhance knowledge of the complex interactions between snow and vegetation. Two field campaigns, during the winters 2016–2017 and 2017–2018, were conducted in a coniferous forest bordering the snow study at Col de Porte (1325 m a.s.l., French Alps) to document the snow accumulation and ablation processes. This paper presents the field site, the instrumentation and the collection and postprocessing methods. The observations include distributed forest characteristics (tree inventory, lidar measurements of forest structure, subcanopy hemispherical photographs), meteorology (automatic weather station and an array of radiometers), snow cover and depth (snow pole transect and laser scan) and snow interception by the canopy during precipitation events. The weather station installed under dense canopy during the first campaign has been maintained since then and has provided continuous measurements throughout the year since 2018. Data are publicly available from the repository of the Observatoire des Sciences de l'Univers de Grenoble (OSUG) data center at https://doi.org/10.17178/SNOUF.2022 (Sicart et al., 2022).

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Earth System Science...arrow_drop_down
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    Earth System Science Data (ESSD)
    Article . 2023 . Peer-reviewed
    License: CC BY
    Data sources: Crossref
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Earth System Science Data (ESSD)
    Other literature type . 2023
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Earth System Science...arrow_drop_down
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Earth System Science Data (ESSD)
      Article . 2023 . Peer-reviewed
      License: CC BY
      Data sources: Crossref
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Earth System Science Data (ESSD)
      Other literature type . 2023
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: S. Lolli; S. Lolli; M. Sicard; M. Sicard; +13 Authors

    Aerosols are one of the most important pollutants in the atmosphere and have been monitored for the past few decades by remote sensing and in situ observation platforms to assess the effectiveness of government-managed reduction emission policies and assess their impact on the radiative budget of the Earth's atmosphere. In fact, aerosols can directly modulate incoming short-wave solar radiation and outgoing long-wave radiation and indirectly influence cloud formation, lifetime, and precipitation. In this study, we quantitatively evaluated long-term temporal trends and seasonal variability from a climatological point of view of the optical and microphysical properties of atmospheric particulate matter at the Universitat Politècnica de Catalunya (UPC), Barcelona, Spain, over the past 17 years, through a synergy of lidar, sun photometer, and in situ concentration measurements. Interannual temporal changes in aerosol optical and microphysical properties are evaluated through the seasonal Mann-Kendall test. Long-term trends in the optical depth of the recovered aerosol; the Ångström exponent (AE); and the concentrations of PM10, PM2.5, and PM1 reveal that emission reduction policies implemented in the past decades were effective in improving air quality, with consistent drops in PM concentrations and optical depth of aerosols. The seasonal analysis of the 17-year average vertically resolved aerosol profiles obtained from lidar observations shows that during summer the aerosol layer can be found up to an altitude of 5 km, after a sharp decay in the first kilometer. In contrast, during the other seasons, the backscatter profiles fit a pronounced exponential decay well with a well-defined scale height. Long-range transport, especially dust outbreaks from the Sahara, is likely to occur throughout the year. During winter, the dust aerosol layers are floating above the boundary layer, while during the other seasons they can penetrate the layer. The analysis also revealed that intense, short-duration pollution events during winter, associated with dust outbreaks, have become more frequent and intense since 2016. This study sheds some light on the meteorological processes and conditions that can lead to the formation of haze and helps decision makers adopt mitigation strategies to preserve large metropolitan areas in the Mediterranean basin. Copyright: This research has been supported by the European Union through NextgenerationEU funds and by the following projects along the years: FP5 EARLINET project (grant no. ID EVR1-CT-1999-40003), FP6 EARLINET-ASOS (ID: 25991), FP7 ACTRIS (ID: 262254), H2020 ACTRIS-2 (ID: 654109), ACTRIS-PPP (ID: 739530), ACTRIS IMP (ID: 871115) and ATMO-ACCESS (ID: 101008004), projects of the Spanish National Research programs (grant nos. TIC 431/93, AMB96-1144-C02-01, REN2000-1907-CE, REN2000-1754-C02-02/CLI, REN2003-09753-C02-C02/CLI, REN2003-09753-C02-C CGL2008-01330-E/CLI 02/CLI, REN2002-12784-E, CGL2005-5131-E, CGL2006-27108-E/CLI, CGL2006-26149-E/CLI, CGL2007-28871-/CLI, CTM2006-27154-E/TECNO, TEC2006-07850/TCM, TEC2009-09106, TEC2012-34575, TEC2015-63832-P and PID2019-103886RB-I00), the project of the Catalan Regional Government IMMPACTE, and the ESA project (grant no. 21487/08/NL/HE). Peer reviewed

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ CNR ExploRAarrow_drop_down
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    CNR ExploRA
    Article . 2023
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    UPCommons. Portal del coneixement obert de la UPC
    Other literature type . Article . 2023 . Peer-reviewed
    License: CC BY
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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    Atmospheric Chemistry and Physics (ACP)
    Article . 2023 . Peer-reviewed
    License: CC BY
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    DIGITAL.CSIC
    Article . 2023 . Peer-reviewed
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      UPCommons. Portal del coneixement obert de la UPC
      Other literature type . Article . 2023 . Peer-reviewed
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      Atmospheric Chemistry and Physics (ACP)
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    Authors: K. Benzerara; A. Elmaleh; M. Ciobanu; A. De Wever; +12 Authors

    Iron and manganese are poorly soluble elements in oxic and alkaline solutions, whereas they are much more soluble under anoxic conditions. As a result, the formation of authigenic mineral phases rich in Fe and/or Mn has traditionally been viewed as diagnostic of global or local anoxic conditions. Here we reveal that some specific cyanobacteria of very small size (< 2 µm, i.e., picocyanobacteria) can biomineralize abundant, authigenic Fe(III)-, Mn(IV)- and Si-rich amorphous phases under oxic conditions in an alkaline lake in Mexico. The resulting biominerals cluster as small globules arranged as rings around the division septum of cyanobacterial cells. These rings are enveloped within an organic, likely polysaccharidic envelope and are partially preserved, at least morphologically, upon sedimentation. Based on their 16S rDNA sequence, these cyanobacteria were affiliated with the Synechococcales order. The high Fe and Mn enrichment of the biominerals questions the systematic inference of anoxic conditions based on their detection. Moreover, this process scavenges iron from the water column, an overlooked biological contribution to the Fe cycle. Finally, it reveals a new case of controlled biomineralization of Si-rich phases by bacteria.

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    Biogeosciences
    Article . 2023 . Peer-reviewed
    License: CC BY
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    Biogeosciences (BG)
    Other literature type . 2023
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      Biogeosciences
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    Authors: X. Shang; A. Lipponen; M. Filioglou; A.-M. Sundström; +12 Authors

    Abstract. In May–June 2019, smoke plumes from wildfires in Alberta, Canada, were advected all the way to Europe. To analyze the evolution of the plumes and to estimate the amount of smoke aerosols transported to Europe, retrievals from the space-borne lidar CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) were used. The plumes were located with the help of a trajectory analysis, and the mass of smoke aerosols were retrieved from the CALIOP observations. The accuracy of the CALIOP mass retrievals was compared with the accuracy of ground-based lidars/ceilometer near the source in North America and after the long-range transport in Europe. Overall, CALIOP and the ground-based lidars/ceilometer produced comparable results. Over North America the CALIOP layer mean mass was 30 % smaller than the ground-based estimates, whereas over Southern Europe that difference varied between 12 % and 43 %. Finally, the CALIOP mass retrievals were compared with simulated aerosol concentrations from two reanalysis models, MERRA-2 (Modern-Era Retrospective analysis for Research and Applications, Version 2) and CAMS (Copernicus Atmospheric Monitoring System). The simulated total column aerosol optical depths (AOD) and the total column mass concentration of smoke agreed quite well with CALIOP observations, but the comparison of the layer mass concentration of smoke showed significant discrepancies. The amount of smoke aerosols in the model simulations was consistently smaller than in the CALIOP retrievals. These results highlight the limitations of such models, and more specifically their limitation to reproduce properly the smoke vertical distribution. They indicate that CALIOP is a useful tool monitoring smoke plumes over secluded areas whereas reanalysis models have difficulties in representing the aerosol mass in these plumes. This study shows the advantages of space-borne aerosol lidars, e.g. being of paramount importance to monitor smoke plumes, and reveals the urgent need of future lidar missions in space.

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    Authors: Salgueiro, V.; Guerrero-Rascado, J.L.; Costa, M.J.; Román, R.; +27 Authors

    Three volcanic plumes were detected during the Tajogaite volcano eruptive activity (Canary Islands, Spain, September–December 2021) over the Iberian Peninsula. The spatiotemporal evolution of these events is characterised by combining passive satellite remote sensing and ground-based lidar and sun-photometer systems. The inversion algorithm GRASP is used with a suite of ground-based remote sensing instruments such as lidar/ceilometer and sun-photometer from eight sites at different locations throughout the Iberian Peninsula. Satellite observations showed that the volcanic ash plumes remained nearby the Canary Islands covering a mean area of 120 ± 202 km2 during the whole period of eruptive activity and that sulphur dioxide plumes reached the Iberian Peninsula. Remote sensing observations showed that the three events were mainly composed of sulphates, which were transported from the volcano into the free troposphere. The high backscatter-related Ångström exponents for wavelengths 532–1064 nm (1.17 ± 0.20 to 1.40 ± 0.24) and low particle depolarization ratios (0.08 ± 0.02 to 0.09 ± 0.02), measured by the multi-wavelength Raman lidar, hinted at the presence of spherical small particles. The layer aerosol optical depth at 532 nm (AODL532) obtained from lidar measurements contributed between 49% and 82% to the AERONET total column AOD at 532 nm in event II (11–13 October). According to the GRASP retrievals, the layer aerosol optical depth at 440 nm (AODL440) was higher in all sites during event II with values between 0.097 (Badajoz) and 0.233 (Guadiana-UGR) and lower in event III (19–21 October) varying between 0.003 (Granada) and 0.026 (Évora). Compared with the GRASP retrievals of total column AOD at 440 nm, the AODL440 had contributions between 21% and 52% during event II. In the event I (25–28 September), the mean volume concentrations (VC) varied between 5 ± 4 μm3cm−3 (El-Arenosillo/Huelva) and 17 ± 10 μm3cm−3 (Guadiana-UGR), while in event II this variation was from 11 ± 7 μm3cm−3 (Badajoz) to 27 ± 10 μm3cm−3 (Guadiana-UGR). Due to the impact of volcanic events on atmospheric and economic fields, such as radiative forcing and airspace security, a proper characterization is required. This work undertakes it using advanced instrumentation and methods. National funds through FCT -Fundacao para a Ciencia e Tecnologia, I.P., in the framework of the ICT project UIDB/04683/2020 UIDP/04683/2020 PROBE Cost Action - NASA Ra-diation Sciences Program and Earth Observing System UIDB/04683/2020 Andalusia Autonomous Government projects AEROPRE and ADAPNE P18-RT-3820 P20_00136 University of Granada Plan Propio through Singular Laboratory LS2022-1 Spanish Government PID2019-103886RB-I00/AEI/10.13039/501100011033 EUMETNET through the E-PROFILE program and REALISTIC 101086690 Scientific Units of Excellence Program RTI 2018-097332-B-C22 CAMELIA PID2019-104205GB- C21/AEI/10.13039/501100011033 NTEGRATYON3 PID2020-117825GB-C21 PID2020-117825GB- C22 INTA predoctoral contract program A-RNM-430-UGR20 UGR-FEDER projects DEM3TRIOS A-RNM-524-UGR20 R+D+i grant MCIN/AEI/ 10.13039/ 501100011033 ACTRIS-Espa ~na CGL2017- 90884REDT TOMA-QAPA PTDC/CTAMET/29678/2017 EPOLAAR RTI2018-097864-B-I00 ERDF A Way of Doing Europe ELPIS PID2020-120015RB-I00 MOGATRACO UCE-PP2017-02 CLARIN CGL2016-81092-R ATMO-ACCESS 101008004 ACTRIS-IMP 871115 GRASP-ACE 778349 HARMONIA CA21119 ACTRIS-2 654109 PROBE CA18235

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    Authors: Marie-Adèle Magnaldo; Quentin Libois; Sébastien Riette; Christine Lac;

    With the worldwide development of the solar energy sector, the need for reliable surface shortwave downward radiation (SWD) forecasts has significantly increased in recent years. SWD forecasts of a few hours to a few days based on numerical weather prediction (NWP) models are essential to facilitate the incorporation of solar energy into the electric grid and ensure network stability. However, SWD errors in NWP models can be substantial. In order to characterize the performances of AROME in detail, the operational NWP model of the French weather service Météo-France, a full year of hourly AROME forecasts is compared to corresponding in situ SWD measurements from 168 high-quality pyranometers covering France. In addition, to classify cloud scenes at high temporal frequency and over the whole territory, cloud products derived from the Satellite Application Facility for Nowcasting and Very Short Range Forecasting (SAF NWC) from geostationary satellites are also used. The 2020 mean bias is positive, with a value of 18 W m−2, meaning that AROME on average overestimates the SWD. The root-mean-square error is 98 W m−2. The situations that contribute the most to the bias correspond to cloudy skies in the model and in the observations, situations that are very frequent (66 %) and characterized by an annual bias of 24 W m−2. Part of this positive bias probably comes from an underestimation of cloud fraction in AROME, although this is not fully addressed in this study due to the lack of consistent observations at kilometer resolution. The other situations have less impact on SWD errors. Missed cloudy situations and erroneously predicted clouds, which generally correspond to clouds with a low impact on the SWD, also have low occurrence (4 % and 11 %). Likewise, well-predicted clear-sky conditions are characterized by a low bias (3 W m−2). When limited to overcast situations in the model, the bias in cloudy skies is small (1 W m−2) but results from large compensating errors. Indeed, further investigation shows that high clouds are systematically associated with a SWD positive bias, while low clouds are associated with a negative bias. This detailed analysis shows that the errors result from a combination of incorrect cloud optical properties and cloud fraction errors, highlighting the need for a more detailed evaluation of cloud properties. This study also provides valuable insights into the potential improvement of AROME physical parametrizations.

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    https://doi.org/10.5194/egusph...
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      https://doi.org/10.5194/egusph...
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    Authors: Mon, Alba; Samper, Javier; Montenegro, Luis; Turrero, María Jesús; +4 Authors

    Carbon steel and compacted bentonite have been proposed as candidate materials for the overpack and buffer, respectively, of the multi-barrier system of a geological high-level radioactive waste repository. Carbon steel corrosion may impair bentonite properties. The interactions of corrosion products and bentonite are analyzed with laboratory corrosion tests. Here coupled thermo-hydro-chemical-mechanical (THCM) models of two types of heating and hydration tests performed on compacted bentonite in contact with Fe powder are presented to study the iron-bentonite interactions at representative repository conditions. Tests on small cells (SC) were performed under unsaturated non-isothermal conditions in 25 mm long columns containing 21 mm of bentonite and 4 mm of Fe powder. Tests on medium-size cells (FB) were performed under unsaturated non-isothermal conditions in 99.8 mm long columns containing 86.8 mm of bentonite and 13 mm of Fe powder. Model results for the SC tests showed that magnetite and Fe(OH)2(s) were the main corrosion products which compete for Fe2+ precipitation. Computed corrosion products precipitate mainly in the Fe powder, penetrate a few mm into the bentonite and reproduce the measured iron weight data. Model results of the FB tests showed that magnetite precipitates throughout the Fe powder interface and reproduce the main trends of the corrosion products. Model results of these corrosion tests will be of great relevance for the performance assessment of engineered barriers of radioactive waste repositories The research leading to these results was funded by ENRESA within the Work Package ACED of EURAD (European Joint Programme on Radioactive Waste Management of the European Union, grant agreement nº 847593), the Spanish Ministry of Science and Innovation (PID2019-109544RB-I00) and the Galician Regional Government (Grant ED431C2021/54). The comments and corrections of the special editor and the two anonymous reviewers are greatly appreciated

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    Biblos-e Archivo; Applied Clay Science
    Other literature type . Article . 2023 . Peer-reviewed
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      Biblos-e Archivo; Applied Clay Science
      Other literature type . Article . 2023 . Peer-reviewed
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    Authors: A. Comerón; C. Muñoz-Porcar; A. Rodríguez-Gómez; M. Sicard; +6 Authors

    We derive an explicit (i.e., non-iterative) formula for the retrieval of the overlap function in an aerosol lidar with both elastic and Raman N2 and/or O2 channels used for independent measurements of aerosol backscatter and extinction coefficients. The formula requires only the measured, range-corrected elastic and the corresponding Raman signals, plus an assumed lidar ratio. We assess the influence of the lidar ratio error in the overlap function retrieval and present retrieval examples. This research has been supported by the Agencia Estatal de Investigación (grant no. PID2019-103886RB-I00) as well as the H2020 Environment (grant nos. 871115 and 101008004) and the H2020 Excellent Science (grant no. 778349) programs. Peer Reviewed

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    Other literature type . Article . 2023 . Peer-reviewed
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: A. Tsekeri; A. Gialitaki; A. Gialitaki; A. Gialitaki; +55 Authors

    Abstract. The European Aerosol Research Lidar Network (EARLINET), part of the Aerosols, Clouds and Trace gases Research Infrastructure (ACTRIS), organized an intensive observational campaign in May 2020, with the objective of monitoring the atmospheric state over Europe during the COVID-19 lockdown and relaxation period. Besides the standard operational processing of the lidar data in EARLINET, for seven EARLINET sites having collocated sun-photometric observations in the Aerosol Robotic Network (AERONET), a network exercise was held in order to derive profiles of the concentration and effective column size distributions of the aerosols in the atmosphere, by applying the GRASP/GARRLiC (from Generalized Aerosol Retrieval from Radiometer and Lidar Combined data – GARRLiC – part of the Generalized Retrieval of Atmosphere and Surface Properties – GRASP) inversion algorithm. The objective of this network exercise was to explore the possibility of identifying the anthropogenic component and of monitoring its spatial and temporal characteristics in the COVID-19 lockdown and relaxation period. While the number of cases is far from being statistically significant so as to provide a conclusive description of the atmospheric aerosols over Europe during this period, this network exercise was fundamental to deriving a common methodology for applying GRASP/GARRLiC to a network of instruments with different characteristics. The limits of the approach are discussed, in particular the missing information close to the ground in the lidar measurements due to the instrument geometry and the sensitivity of the GRASP/GARRLiC retrieval to the settings used, especially for cases with low aerosol optical depth (AOD) like the ones we show here. We found that this sensitivity is well-characterized in the GRASP/GARRLiC products, since it is included in their retrieval uncertainties.

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    Atmospheric Measurement Techniques
    Article . 2023 . Peer-reviewed
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      Atmospheric Measurement Techniques
      Article . 2023 . Peer-reviewed
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    Authors: Rémy Ballot; Nicolas Guilpart; Marie-Hélène Jeuffroy;

    Crop diversification is considered a key element of agroecological transition, whereas current dominant cropping systems are known to rely on only a few crop species – like cereals in Europe. To assess the benefits of crop diversification at a large scale, an accurate description of current crop sequences is required as a baseline. However, such a description is lacking at the scale of Europe. Here, we developed the first map of dominant crop sequences in Europe for the period 2012–2018. We used the Land Use Cover Area frame statistical Survey (LUCAS) dataset that provides temporally incomplete (2012, 2015 and 2018) land cover information from a stable grid of points covering Europe. Eight crop sequence types were identified using hierarchical clustering implemented on LUCAS data and mapped over Europe. We show, in France, that the relative importance of these eight crop sequence types (as estimated from LUCAS data) was highly consistent with those derived from an almost spatially exhaustive temporally complete national dataset (the French Land Parcel Identification System) for the same period, thus validating the method and typology for this country. Land use (i.e. crop production area) derived from our map of dominant crop sequences was also highly consistent with land use reported by official statistics at both national and European levels, validating the approach at a European scale. This first map of dominant crop sequences in Europe should be useful for future studies dealing with agricultural issues that are sensitive to crop rotations. The map of dominant crop sequence types in Europe derived from our work is available at https://doi.org/10.5281/zenodo.7016986 (Ballot et al., 2022).

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    Earth System Science Data (ESSD)
    Article . 2023 . Peer-reviewed
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      Earth System Science Data (ESSD)
      Article . 2023 . Peer-reviewed
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    Authors: Sicart, Jean Emmanuel; Ramseyer, Victor; Picard, Ghislain; Arnaud, Laurent; +15 Authors

    Forests strongly modify the accumulation, metamorphism and melting of snow in midlatitude and high-latitude regions. Recently, snow routines in hydrological and land surface models were improved to incorporate more accurate representations of forest snow processes, but model intercomparison projects have identified deficiencies, partly due to incomplete knowledge of the processes controlling snow cover in forests. The Snow Under Forest (SnoUF) project was initiated to enhance knowledge of the complex interactions between snow and vegetation. Two field campaigns, during the winters 2016–2017 and 2017–2018, were conducted in a coniferous forest bordering the snow study at Col de Porte (1325 m a.s.l., French Alps) to document the snow accumulation and ablation processes. This paper presents the field site, the instrumentation and the collection and postprocessing methods. The observations include distributed forest characteristics (tree inventory, lidar measurements of forest structure, subcanopy hemispherical photographs), meteorology (automatic weather station and an array of radiometers), snow cover and depth (snow pole transect and laser scan) and snow interception by the canopy during precipitation events. The weather station installed under dense canopy during the first campaign has been maintained since then and has provided continuous measurements throughout the year since 2018. Data are publicly available from the repository of the Observatoire des Sciences de l'Univers de Grenoble (OSUG) data center at https://doi.org/10.17178/SNOUF.2022 (Sicart et al., 2022).

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    Earth System Science Data (ESSD)
    Article . 2023 . Peer-reviewed
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      Earth System Science Data (ESSD)
      Article . 2023 . Peer-reviewed
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: S. Lolli; S. Lolli; M. Sicard; M. Sicard; +13 Authors

    Aerosols are one of the most important pollutants in the atmosphere and have been monitored for the past few decades by remote sensing and in situ observation platforms to assess the effectiveness of government-managed reduction emission policies and assess their impact on the radiative budget of the Earth's atmosphere. In fact, aerosols can directly modulate incoming short-wave solar radiation and outgoing long-wave radiation and indirectly influence cloud formation, lifetime, and precipitation. In this study, we quantitatively evaluated long-term temporal trends and seasonal variability from a climatological point of view of the optical and microphysical properties of atmospheric particulate matter at the Universitat Politècnica de Catalunya (UPC), Barcelona, Spain, over the past 17 years, through a synergy of lidar, sun photometer, and in situ concentration measurements. Interannual temporal changes in aerosol optical and microphysical properties are evaluated through the seasonal Mann-Kendall test. Long-term trends in the optical depth of the recovered aerosol; the Ångström exponent (AE); and the concentrations of PM10, PM2.5, and PM1 reveal that emission reduction policies implemented in the past decades were effective in improving air quality, with consistent drops in PM concentrations and optical depth of aerosols. The seasonal analysis of the 17-year average vertically resolved aerosol profiles obtained from lidar observations shows that during summer the aerosol layer can be found up to an altitude of 5 km, after a sharp decay in the first kilometer. In contrast, during the other seasons, the backscatter profiles fit a pronounced exponential decay well with a well-defined scale height. Long-range transport, especially dust outbreaks from the Sahara, is likely to occur throughout the year. During winter, the dust aerosol layers are floating above the boundary layer, while during the other seasons they can penetrate the layer. The analysis also revealed that intense, short-duration pollution events during winter, associated with dust outbreaks, have become more frequent and intense since 2016. This study sheds some light on the meteorological processes and conditions that can lead to the formation of haze and helps decision makers adopt mitigation strategies to preserve large metropolitan areas in the Mediterranean basin. Copyright: This research has been supported by the European Union through NextgenerationEU funds and by the following projects along the years: FP5 EARLINET project (grant no. ID EVR1-CT-1999-40003), FP6 EARLINET-ASOS (ID: 25991), FP7 ACTRIS (ID: 262254), H2020 ACTRIS-2 (ID: 654109), ACTRIS-PPP (ID: 739530), ACTRIS IMP (ID: 871115) and ATMO-ACCESS (ID: 101008004), projects of the Spanish National Research programs (grant nos. TIC 431/93, AMB96-1144-C02-01, REN2000-1907-CE, REN2000-1754-C02-02/CLI, REN2003-09753-C02-C02/CLI, REN2003-09753-C02-C CGL2008-01330-E/CLI 02/CLI, REN2002-12784-E, CGL2005-5131-E, CGL2006-27108-E/CLI, CGL2006-26149-E/CLI, CGL2007-28871-/CLI, CTM2006-27154-E/TECNO, TEC2006-07850/TCM, TEC2009-09106, TEC2012-34575, TEC2015-63832-P and PID2019-103886RB-I00), the project of the Catalan Regional Government IMMPACTE, and the ESA project (grant no. 21487/08/NL/HE). Peer reviewed

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    Other literature type . Article . 2023 . Peer-reviewed
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    Atmospheric Chemistry and Physics (ACP)
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    Authors: K. Benzerara; A. Elmaleh; M. Ciobanu; A. De Wever; +12 Authors

    Iron and manganese are poorly soluble elements in oxic and alkaline solutions, whereas they are much more soluble under anoxic conditions. As a result, the formation of authigenic mineral phases rich in Fe and/or Mn has traditionally been viewed as diagnostic of global or local anoxic conditions. Here we reveal that some specific cyanobacteria of very small size (< 2 µm, i.e., picocyanobacteria) can biomineralize abundant, authigenic Fe(III)-, Mn(IV)- and Si-rich amorphous phases under oxic conditions in an alkaline lake in Mexico. The resulting biominerals cluster as small globules arranged as rings around the division septum of cyanobacterial cells. These rings are enveloped within an organic, likely polysaccharidic envelope and are partially preserved, at least morphologically, upon sedimentation. Based on their 16S rDNA sequence, these cyanobacteria were affiliated with the Synechococcales order. The high Fe and Mn enrichment of the biominerals questions the systematic inference of anoxic conditions based on their detection. Moreover, this process scavenges iron from the water column, an overlooked biological contribution to the Fe cycle. Finally, it reveals a new case of controlled biomineralization of Si-rich phases by bacteria.

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    Biogeosciences
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      Biogeosciences
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    Authors: X. Shang; A. Lipponen; M. Filioglou; A.-M. Sundström; +12 Authors

    Abstract. In May–June 2019, smoke plumes from wildfires in Alberta, Canada, were advected all the way to Europe. To analyze the evolution of the plumes and to estimate the amount of smoke aerosols transported to Europe, retrievals from the space-borne lidar CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) were used. The plumes were located with the help of a trajectory analysis, and the mass of smoke aerosols were retrieved from the CALIOP observations. The accuracy of the CALIOP mass retrievals was compared with the accuracy of ground-based lidars/ceilometer near the source in North America and after the long-range transport in Europe. Overall, CALIOP and the ground-based lidars/ceilometer produced comparable results. Over North America the CALIOP layer mean mass was 30 % smaller than the ground-based estimates, whereas over Southern Europe that difference varied between 12 % and 43 %. Finally, the CALIOP mass retrievals were compared with simulated aerosol concentrations from two reanalysis models, MERRA-2 (Modern-Era Retrospective analysis for Research and Applications, Version 2) and CAMS (Copernicus Atmospheric Monitoring System). The simulated total column aerosol optical depths (AOD) and the total column mass concentration of smoke agreed quite well with CALIOP observations, but the comparison of the layer mass concentration of smoke showed significant discrepancies. The amount of smoke aerosols in the model simulations was consistently smaller than in the CALIOP retrievals. These results highlight the limitations of such models, and more specifically their limitation to reproduce properly the smoke vertical distribution. They indicate that CALIOP is a useful tool monitoring smoke plumes over secluded areas whereas reanalysis models have difficulties in representing the aerosol mass in these plumes. This study shows the advantages of space-borne aerosol lidars, e.g. being of paramount importance to monitor smoke plumes, and reveals the urgent need of future lidar missions in space.

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    https://doi.org/10.5194/egusph...
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      https://doi.org/10.5194/egusph...
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    Authors: Salgueiro, V.; Guerrero-Rascado, J.L.; Costa, M.J.; Román, R.; +27 Authors

    Three volcanic plumes were detected during the Tajogaite volcano eruptive activity (Canary Islands, Spain, September–December 2021) over the Iberian Peninsula. The spatiotemporal evolution of these events is characterised by combining passive satellite remote sensing and ground-based lidar and sun-photometer systems. The inversion algorithm GRASP is used with a suite of ground-based remote sensing instruments such as lidar/ceilometer and sun-photometer from eight sites at different locations throughout the Iberian Peninsula. Satellite observations showed that the volcanic ash plumes remained nearby the Canary Islands covering a mean area of 120 ± 202 km2 during the whole period of eruptive activity and that sulphur dioxide plumes reached the Iberian Peninsula. Remote sensing observations showed that the three events were mainly composed of sulphates, which were transported from the volcano into the free troposphere. The high backscatter-related Ångström exponents for wavelengths 532–1064 nm (1.17 ± 0.20 to 1.40 ± 0.24) and low particle depolarization ratios (0.08 ± 0.02 to 0.09 ± 0.02), measured by the multi-wavelength Raman lidar, hinted at the presence of spherical small particles. The layer aerosol optical depth at 532 nm (AODL532) obtained from lidar measurements contributed between 49% and 82% to the AERONET total column AOD at 532 nm in event II (11–13 October). According to the GRASP retrievals, the layer aerosol optical depth at 440 nm (AODL440) was higher in all sites during event II with values between 0.097 (Badajoz) and 0.233 (Guadiana-UGR) and lower in event III (19–21 October) varying between 0.003 (Granada) and 0.026 (Évora). Compared with the GRASP retrievals of total column AOD at 440 nm, the AODL440 had contributions between 21% and 52% during event II. In the event I (25–28 September), the mean volume concentrations (VC) varied between 5 ± 4 μm3cm−3 (El-Arenosillo/Huelva) and 17 ± 10 μm3cm−3 (Guadiana-UGR), while in event II this variation was from 11 ± 7 μm3cm−3 (Badajoz) to 27 ± 10 μm3cm−3 (Guadiana-UGR). Due to the impact of volcanic events on atmospheric and economic fields, such as radiative forcing and airspace security, a proper characterization is required. This work undertakes it using advanced instrumentation and methods. National funds through FCT -Fundacao para a Ciencia e Tecnologia, I.P., in the framework of the ICT project UIDB/04683/2020 UIDP/04683/2020 PROBE Cost Action - NASA Ra-diation Sciences Program and Earth Observing System UIDB/04683/2020 Andalusia Autonomous Government projects AEROPRE and ADAPNE P18-RT-3820 P20_00136 University of Granada Plan Propio through Singular Laboratory LS2022-1 Spanish Government PID2019-103886RB-I00/AEI/10.13039/501100011033 EUMETNET through the E-PROFILE program and REALISTIC 101086690 Scientific Units of Excellence Program RTI 2018-097332-B-C22 CAMELIA PID2019-104205GB- C21/AEI/10.13039/501100011033 NTEGRATYON3 PID2020-117825GB-C21 PID2020-117825GB- C22 INTA predoctoral contract program A-RNM-430-UGR20 UGR-FEDER projects DEM3TRIOS A-RNM-524-UGR20 R+D+i grant MCIN/AEI/ 10.13039/ 501100011033 ACTRIS-Espa ~na CGL2017- 90884REDT TOMA-QAPA PTDC/CTAMET/29678/2017 EPOLAAR RTI2018-097864-B-I00 ERDF A Way of Doing Europe ELPIS PID2020-120015RB-I00 MOGATRACO UCE-PP2017-02 CLARIN CGL2016-81092-R ATMO-ACCESS 101008004 ACTRIS-IMP 871115 GRASP-ACE 778349 HARMONIA CA21119 ACTRIS-2 654109 PROBE CA18235

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    Authors: Marie-Adèle Magnaldo; Quentin Libois; Sébastien Riette; Christine Lac;

    With the worldwide development of the solar energy sector, the need for reliable surface shortwave downward radiation (SWD) forecasts has significantly increased in recent years. SWD forecasts of a few hours to a few days based on numerical weather prediction (NWP) models are essential to facilitate the incorporation of solar energy into the electric grid and ensure network stability. However, SWD errors in NWP models can be substantial. In order to characterize the performances of AROME in detail, the operational NWP model of the French weather service Météo-France, a full year of hourly AROME forecasts is compared to corresponding in situ SWD measurements from 168 high-quality pyranometers covering France. In addition, to classify cloud scenes at high temporal frequency and over the whole territory, cloud products derived from the Satellite Application Facility for Nowcasting and Very Short Range Forecasting (SAF NWC) from geostationary satellites are also used. The 2020 mean bias is positive, with a value of 18 W m−2, meaning that AROME on average overestimates the SWD. The root-mean-square error is 98 W m−2. The situations that contribute the most to the bias correspond to cloudy skies in the model and in the observations, situations that are very frequent (66 %) and characterized by an annual bias of 24 W m−2. Part of this positive bias probably comes from an underestimation of cloud fraction in AROME, although this is not fully addressed in this study due to the lack of consistent observations at kilometer resolution. The other situations have less impact on SWD errors. Missed cloudy situations and erroneously predicted clouds, which generally correspond to clouds with a low impact on the SWD, also have low occurrence (4 % and 11 %). Likewise, well-predicted clear-sky conditions are characterized by a low bias (3 W m−2). When limited to overcast situations in the model, the bias in cloudy skies is small (1 W m−2) but results from large compensating errors. Indeed, further investigation shows that high clouds are systematically associated with a SWD positive bias, while low clouds are associated with a negative bias. This detailed analysis shows that the errors result from a combination of incorrect cloud optical properties and cloud fraction errors, highlighting the need for a more detailed evaluation of cloud properties. This study also provides valuable insights into the potential improvement of AROME physical parametrizations.

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    https://doi.org/10.5194/egusph...
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      https://doi.org/10.5194/egusph...
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    Authors: Mon, Alba; Samper, Javier; Montenegro, Luis; Turrero, María Jesús; +4 Authors

    Carbon steel and compacted bentonite have been proposed as candidate materials for the overpack and buffer, respectively, of the multi-barrier system of a geological high-level radioactive waste repository. Carbon steel corrosion may impair bentonite properties. The interactions of corrosion products and bentonite are analyzed with laboratory corrosion tests. Here coupled thermo-hydro-chemical-mechanical (THCM) models of two types of heating and hydration tests performed on compacted bentonite in contact with Fe powder are presented to study the iron-bentonite interactions at representative repository conditions. Tests on small cells (SC) were performed under unsaturated non-isothermal conditions in 25 mm long columns containing 21 mm of bentonite and 4 mm of Fe powder. Tests on medium-size cells (FB) were performed under unsaturated non-isothermal conditions in 99.8 mm long columns containing 86.8 mm of bentonite and 13 mm of Fe powder. Model results for the SC tests showed that magnetite and Fe(OH)2(s) were the main corrosion products which compete for Fe2+ precipitation. Computed corrosion products precipitate mainly in the Fe powder, penetrate a few mm into the bentonite and reproduce the measured iron weight data. Model results of the FB tests showed that magnetite precipitates throughout the Fe powder interface and reproduce the main trends of the corrosion products. Model results of these corrosion tests will be of great relevance for the performance assessment of engineered barriers of radioactive waste repositories The research leading to these results was funded by ENRESA within the Work Package ACED of EURAD (European Joint Programme on Radioactive Waste Management of the European Union, grant agreement nº 847593), the Spanish Ministry of Science and Innovation (PID2019-109544RB-I00) and the Galician Regional Government (Grant ED431C2021/54). The comments and corrections of the special editor and the two anonymous reviewers are greatly appreciated

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    Biblos-e Archivo; Applied Clay Science
    Other literature type . Article . 2023 . Peer-reviewed
    License: Elsevier TDM
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      Biblos-e Archivo; Applied Clay Science
      Other literature type . Article . 2023 . Peer-reviewed
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    Authors: A. Comerón; C. Muñoz-Porcar; A. Rodríguez-Gómez; M. Sicard; +6 Authors

    We derive an explicit (i.e., non-iterative) formula for the retrieval of the overlap function in an aerosol lidar with both elastic and Raman N2 and/or O2 channels used for independent measurements of aerosol backscatter and extinction coefficients. The formula requires only the measured, range-corrected elastic and the corresponding Raman signals, plus an assumed lidar ratio. We assess the influence of the lidar ratio error in the overlap function retrieval and present retrieval examples. This research has been supported by the Agencia Estatal de Investigación (grant no. PID2019-103886RB-I00) as well as the H2020 Environment (grant nos. 871115 and 101008004) and the H2020 Excellent Science (grant no. 778349) programs. Peer Reviewed

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