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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Victoria Reyes-García; David García-del-Amo; Santiago Álvarez-Fernández; Petra Benyei; +54 Authors

    AbstractThe effects of climate change depend on specific local circumstances, posing a challenge for worldwide research to comprehensively encompass the diverse impacts on various local social-ecological systems. Here we use a place-specific but cross-culturally comparable protocol to document climate change indicators and impacts as locally experienced and analyze their distribution. We collected first-hand data in 48 sites inhabited by Indigenous Peoples and local communities and covering all climate zones and nature-dependent livelihoods. We documented 1,661 site-agreed reports of change corresponding to 369 indicators. Reports of change vary according to climate zone and livelihood activity. We provide compelling evidence that climate change impacts on Indigenous Peoples and local communities are ongoing, tangible, widespread, and affect multiple elements of their social-ecological systems. Beyond potentially informing contextualized adaptation plans, our results show that local reports could help identify economic and non-economic loss and damage related to climate change impacts suffered by Indigenous Peoples and local communities.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ HELDA - Digital Repo...arrow_drop_down
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Research@WUR; Communications Earth & Environment
    Other literature type . Article . 2024 . Peer-reviewed
    License: CC BY
    DOAJ
    Article . 2024
    Data sources: DOAJ
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ HELDA - Digital Repo...arrow_drop_down
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Research@WUR; Communications Earth & Environment
      Other literature type . Article . 2024 . Peer-reviewed
      License: CC BY
      DOAJ
      Article . 2024
      Data sources: DOAJ
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Xiansheng, Liu; Hadiatullah, Hadiatullah; Xun, Zhang; Pedro, Trechera; +48 Authors

    This study is supported by the RI-URBANS project (Research Infrastructures Services Reinforcing Air Quality Monitoring Capacities in European Urban & amp; Industrial Areas, European Union's Horizon 2020 research and innovation program, Green Deal, European Commission, contract 101036245). This study is also supported by National Natural Science Foundation of China (42101470, 72242106) and in part by the Chunhui Project Foundation of the Education Department of China under Grant HZKY20220053. This study benefited from the Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS), especially the so-called ACTRIS-2 H2020 research project (grant no 654109), and the authors would like to thank ACTRIS (The Aerosol, Clouds and Trace Gases Research Infrastructure), especially the ACTRIS in situ EBAS Data Centre (EBAS), for providing datasets to the study. This study is also partly funded by the National Institute for Health Research (NIHR) Health Protection Research Unit in Environmental Exposures and Health, a partnership between UK Health Security Agency (UKHSA) and Imperial College London, and the UK Natural Environment Re-search Council, and the views expressed are those of the author(s) and not necessarily those of the NIHR, UKHSA or the Department of Health and Social Care. The research was also supported by the Hungarian Research, Development and Innovation Office (grant no. K132254). We thank also the support from "Agencia Estatal de Investigacion" from the Spanish Ministry of Science and Innovation, and FEDER funds under the projects CAIAC (PID2019-108990RB-I00); and the Generalitat de Catalunya (AGAUR 2017 SGR41) and the Direccio General de Territori. IMT Nord Europe and LOA acknowledge financial support from the Labex CaPPA project, funded by the French National Research Agency (ANR-11-LABX-0005-01), and the CLIMIBIO and ECRIN projects, both financed by the Regional Council "Hauts-de-France" and the European Regional Development Fund (ERDF). This study aims to picture the phenomenology of urban ambient total lung deposited surface area (LDSA) (including head/throat (HA), tracheobronchial (TB), and alveolar (ALV) regions) based on multiple path particle dosimetry (MPPD) model during 2017-2019 period collected from urban background (UB, n = 15), traffic (TR, n = 6), suburban background (SUB, n = 4), and regional background (RB, n = 1) monitoring sites in Europe (25) and USA (1). Briefly, the spatial-temporal distribution characteristics of the deposition of LDSA, including diel, weekly, and seasonal pat-terns, were analyzed. Then, the relationship between LDSA and other air quality metrics at each monitoring site was investigated. The result showed that the peak concentrations of LDSA at UB and TR sites are commonly observed in the morning (06:00-8:00 UTC) and late evening (19:00-22:00 UTC), coinciding with traffic rush hours, biomass burning, and atmospheric stagnation periods. The only LDSA night-time peaks are observed on weekends. Due to the variability of emission sources and meteorology, the seasonal variability of the LDSA concentration revealed sig-nificant differences (p = 0.01) between the four seasons at all monitoring sites. Meanwhile, the correlations of LDSA with other pollutant metrics suggested that Aitken and accumulation mode particles play a significant role in the total LDSA concentration. The results also indicated that the main proportion of total LDSA is attributed to the ALV fraction (50 %), followed by the TB (34 %) and HA (16 %). Overall, this study provides valuable information of LDSA as a predictor in epidemiological studies and for the first time presenting total LDSA in a variety of European urban environments. RI-URBANS project (Research Infrastructures Services Reinforcing Air Quality Monitoring Capacities in European Urban amp; Industrial Areas, European Union's Horizon 2020 research and innovation program, Green Deal, European Commission, 101036245) National Institute for Health Research (NIHR) Health Protection Research Unit in Environmental Exposures and Health European Union (EU) K132254, PID2019-108990RB-I00, AGAUR 2017 SGR41, ANR-11-LABX-0005-01 "Agencia Estatal de Investigacion" from the Spanish Ministry of Science and Innovation UK Research & Innovation (UKRI) Natural Environment Research Council (NERC) National Research, Development & Innovation Office (NRDIO) - Hungary Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS) Chunhui Project Foundation of the Education Department of China National Natural Science Foundation of China (NSFC) Agence Nationale de la Recherche (ANR) 654109 Generalitat de Catalunya 42101470, 72242106 Direccio General de Territori HZKY20220053 Regional Council "Hauts-de-France" ERDF

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    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
    Lille Open Archive
    Article . 2023
    Data sources: Lille Open Archive
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: M. J. Campmier; J. Gingrich; S. Singh; N. Baig; +12 Authors

    Lower-cost air pollution sensors can fill critical air quality data gaps in India, which experiences very high fine particulate matter (PM2.5) air pollution but has sparse regulatory air monitoring. Challenges for low-cost PM2.5 sensors in India include high-aerosol mass concentrations and pronounced regional and seasonal gradients in aerosol composition. Here, we report on a detailed long-time performance evaluation of a popular sensor, the Purple Air PA-II, at multiple sites in India. We established three distinct sites in India across land use categories and population density extremes (in urban Delhi and rural Hamirpur in north India and urban Bengaluru in south India), where we collocated the PA-II model with reference beta attenuation monitors. We evaluated the performance of uncalibrated sensor data, and then developed, optimized, and evaluated calibration models using a comprehensive feature selection process with a view to reproducibility in the Indian context. We assessed the seasonal and spatial transferability of sensor calibration schemes, which is especially important in India because of the paucity of reference instrumentation. Without calibration, the PA-II was moderately correlated with the reference signal (R2 = 0.55–0.74) but was inaccurate (NRMSE ≥ 40 %). Relative to uncalibrated data, parsimonious annual calibration models improved the PurpleAir (PA) model performance at all sites (cross-validated NRMSE 20 %–30 %; R2 = 0.82–0.95), and greatly reduced seasonal and diurnal biases. Because aerosol properties and meteorology vary regionally, the form of these long-term models differed among our sites, suggesting that local calibrations are desirable when possible. Using a moving-window calibration, we found that using seasonally specific information improves performance relative to a static annual calibration model, while a short-term calibration model generally does not transfer reliably to other seasons. Overall, we find that the PA-II model can provide reliable PM2.5 data with better than ±25 % precision and accuracy when paired with a rigorous calibration scheme that accounts for seasonality and local aerosol composition.

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ HELDA - Digital Repo...arrow_drop_down
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Atmospheric Measurement Techniques
    Article . 2023 . Peer-reviewed
    License: CC BY
    Data sources: Crossref
    DOAJ
    Article . 2023
    Data sources: DOAJ
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ HELDA - Digital Repo...arrow_drop_down
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      Atmospheric Measurement Techniques
      Article . 2023 . Peer-reviewed
      License: CC BY
      Data sources: Crossref
      DOAJ
      Article . 2023
      Data sources: DOAJ
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: M. J. McGrath; A. M. R. Petrescu; P. Peylin; R. M. Andrew; +69 Authors

    Quantification of land surface–atmosphere fluxes of carbon dioxide (CO2) and their trends and uncertainties is essential for monitoring progress of the EU27+UK bloc as it strives to meet ambitious targets determined by both international agreements and internal regulation. This study provides a consolidated synthesis of fossil sources (CO2 fossil) and natural (including formally managed ecosystems) sources and sinks over land (CO2 land) using bottom-up (BU) and top-down (TD) approaches for the European Union and United Kingdom (EU27+UK), updating earlier syntheses (Petrescu et al., 2020, 2021). Given the wide scope of the work and the variety of approaches involved, this study aims to answer essential questions identified in the previous syntheses and understand the differences between datasets, particularly for poorly characterized fluxes from managed and unmanaged ecosystems. The work integrates updated emission inventory data, process-based model results, data-driven categorical model results, and inverse modeling estimates, extending the previous period 1990–2018 to the year 2020 to the extent possible. BU and TD products are compared with the European national greenhouse gas inventory (NGHGI) reported by parties including the year 2019 under the United Nations Framework Convention on Climate Change (UNFCCC). The uncertainties of the EU27+UK NGHGI were evaluated using the standard deviation reported by the EU member states following the guidelines of the Intergovernmental Panel on Climate Change (IPCC) and harmonized by gap-filling procedures. Variation in estimates produced with other methods, such as atmospheric inversion models (TD) or spatially disaggregated inventory datasets (BU), originate from within-model uncertainty related to parameterization as well as structural differences between models. By comparing the NGHGI with other approaches, key sources of differences between estimates arise primarily in activities. System boundaries and emission categories create differences in CO2 fossil datasets, while different land use definitions for reporting emissions from land use, land use change, and forestry (LULUCF) activities result in differences for CO2 land. The latter has important consequences for atmospheric inversions, leading to inversions reporting stronger sinks in vegetation and soils than are reported by the NGHGI. For CO2 fossil emissions, after harmonizing estimates based on common activities and selecting the most recent year available for all datasets, the UNFCCC NGHGI for the EU27+UK accounts for 926 ± 13 Tg C yr−1, while eight other BU sources report a mean value of 948 [937,961] Tg C yr−1 (25th, 75th percentiles). The sole top-down inversion of fossil emissions currently available accounts for 875 Tg C in this same year, a value outside the uncertainty of both the NGHGI and bottom-up ensemble estimates and for which uncertainty estimates are not currently available. For the net CO2 land fluxes, during the most recent 5-year period including the NGHGI estimates, the NGHGI accounted for −91 ± 32 Tg C yr−1, while six other BU approaches reported a mean sink of −62 [-117,-49] Tg C yr−1, and a 15-member ensemble of dynamic global vegetation models (DGVMs) reported −69 [-152,-5] Tg C yr−1. The 5-year mean of three TD regional ensembles combined with one non-ensemble inversion of −73 Tg C yr−1 has a slightly smaller spread (0th–100th percentiles of [-135,+45] Tg C yr−1), and it was calculated after removing net land–atmosphere CO2 fluxes caused by lateral transport of carbon (crop trade, wood trade, river transport, and net uptake from inland water bodies), resulting in increased agreement with the NGHGI and bottom-up approaches. Results at the category level (Forest Land, Cropland, Grassland) generally show good agreement between the NGHGI and category-specific models, but results for DGVMs are mixed. Overall, for both CO2 fossil and net CO2 land fluxes, we find that current independent approaches are consistent with the NGHGI at the scale of the EU27+UK. We conclude that CO2 emissions from fossil sources have decreased over the past 30 years in the EU27+UK, while land fluxes are relatively stable: positive or negative trends larger (smaller) than 0.07 (−0.61) Tg C yr−2 can be ruled out for the NGHGI. In addition, a gap on the order of 1000 Tg C yr−1 between CO2 fossil emissions and net CO2 uptake by the land exists regardless of the type of approach (NGHGI, TD, BU), falling well outside all available estimates of uncertainties. However, uncertainties in top-down approaches to estimate CO2 fossil emissions remain uncharacterized and are likely substantial, in addition to known uncertainties in top-down estimates of the land fluxes. The data used to plot the figures are available at https://doi.org/10.5281/zenodo.8148461 (McGrath et al., 2023).

    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ University of East A...arrow_drop_down
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    MPG.PuRe
    Article . 2023
    Data sources: MPG.PuRe
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    MPG.PuRe
    Article . 2023
    License: CC BY
    Data sources: MPG.PuRe
    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Earth System Science Data (ESSD)
    Other literature type . 2023
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    NILU Brage
    Article . 2023
    Data sources: NILU Brage
    DOAJ
    Article . 2023
    Data sources: DOAJ
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ University of East A...arrow_drop_down
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      MPG.PuRe
      Article . 2023
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      MPG.PuRe
      Article . 2023
      License: CC BY
      Data sources: MPG.PuRe
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      Earth System Science Data (ESSD)
      Other literature type . 2023
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      NILU Brage
      Article . 2023
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      DOAJ
      Article . 2023
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    Authors: M. Räsänen; R. Vesala; P. Rönnholm; L. Arppe; +8 Authors

    Termites play an essential role in decomposing dead plant material in tropical ecosystems and are thus major sources of gaseous C emissions in many environments. In African savannas, fungus-growing termites are among the ecologically most influential termite species. We studied the gas exchange from mounds of two closely related fungus-growing species (Macrotermes subhyalinus and M. michaelseni, respectively) in two habitats representing different vegetation types (grassland, bushland) together with soil fluxes around the mounds. The fluxes from active termite mounds varied from 120 to 2100 mg CO2–C m−2 h−1 for carbon dioxide (CO2) and from 0.06 to 3.7 mg CH4–C m−2 h−1 for methane (CH4) fluxes. Mound CO2 fluxes varied seasonally with a 64 % decrease and 41 % increase in the fluxes from the dry to wet season at the grassland and bushland sites, respectively. During the wet season, the CO2 fluxes were significantly correlated with termite mound volume. The diurnal measurements from two M. michaelseni mounds suggest that the gas fluxes peak during the daytime, possibly reflecting changes in mound internal air circulation. Soil fluxes of both CO2 and CH4 were enhanced at up to 2 m distance from the mounds compared to the local soil respiration, indicating that, in addition to mound ventilation structures, a small proportion of the metabolic gases produced also leave the nest via surrounding soils.

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    Biogeosciences (BG)
    Other literature type . 2023
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    Aaltodoc Publication Archive
    Article . 2023 . Peer-reviewed
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    Biogeosciences
    Article . 2023 . Peer-reviewed
    License: CC BY
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    DOAJ
    Article . 2023
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      Biogeosciences (BG)
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      Aaltodoc Publication Archive
      Article . 2023 . Peer-reviewed
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      Biogeosciences
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      DOAJ
      Article . 2023
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    Authors: Lubna Dada; Dominik Stolzenburg; Mario Simon; Lukas Fischer; +51 Authors

    Biogenic vapors form new particles in the atmosphere, affecting global climate. The contributions of monoterpenes and isoprene to new particle formation (NPF) have been extensively studied. However, sesquiterpenes have received little attention despite a potentially important role due to their high molecular weight. Via chamber experiments performed under atmospheric conditions, we report biogenic NPF resulting from the oxidation of pure mixtures of beta-caryophyllene, alpha-pinene, and isoprene, which produces oxygenated compounds over a wide range of volatilities. We find that a class of vapors termed ultralow-volatility organic compounds (ULVOCs) are highly efficient nucleators and quantitatively determine NPF efficiency. When compared with a mixture of isoprene and monoterpene alone, adding only 2% sesquiterpene increases the ULVOC yield and doubles the formation rate. Thus, sesquiterpene emissions need to be included in assessments of global aerosol concentrations in pristine climates where biogenic NPF is expected to be a major source of cloud condensation nuclei. Peer reviewed

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    Science Advances
    Article . 2023 . Peer-reviewed
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    KITopen
    Article . 2023
    License: CC BY NC
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    https://doi.org/10.5445/ir/100...
    Article . 2023
    License: CC BY NC
    Data sources: Datacite
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    CERN Document Server
    Other literature type . 2023
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    Science Advances
    Article . 2023
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      Science Advances
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      KITopen
      Article . 2023
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      https://doi.org/10.5445/ir/100...
      Article . 2023
      License: CC BY NC
      Data sources: Datacite
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      CERN Document Server
      Other literature type . 2023
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      Science Advances
      Article . 2023
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    Authors: A. Zanchetta; L. M. J. Kooijmans; L. M. J. Kooijmans; S. van Heuven; +9 Authors

    Carbonyl sulfide (COS) is a promising tracer for the estimation of terrestrial ecosystem gross primary production (GPP). However, understanding its non-GPP-related sources and sinks, e.g., anthropogenic sources and soil sources and sinks, is also critical to the success of the approach. Here we infer the regional sources and sinks of COS using continuous in situ mole fraction profile measurements of COS along the 60 m tall Lutjewad tower (1 m a.s.l.; 53∘24′ N, 6∘21′ E) in the Netherlands. To identify potential sources that caused the observed enhancements of COS mole fractions at Lutjewad, both discrete flask samples and in situ measurements in the province of Groningen were made from a mobile van using a quantum cascade laser spectrometer (QCLS). We also simulated the COS mole fractions at Lutjewad using the Stochastic Time-Inverted Lagrangian Transport (STILT) model combined with emission inventories and plant uptake fluxes. We determined the nighttime COS fluxes to be -3.0±2.6 pmol m−2 s−1 using the radon-tracer correlation approach and Lutjewad observations. Furthermore, we identified and quantified several COS sources, including biodigesters, sugar production facilities and silicon carbide production facilities in the province of Groningen. Moreover, the simulation results show that the observed COS enhancements can be partially explained by known industrial sources of COS and CS2, in particular from the Ruhr Valley (51.5∘ N, 7.2∘ E) and Antwerp (51.2∘ N, 4.4∘ E) areas. The contribution of likely missing anthropogenic sources of COS and CS2 in the inventory may be significant. The impact of the identified sources in the province of Groningen is estimated to be negligible in terms of the observed COS enhancements. However, in specific conditions, these sources may influence the measurements in Lutjewad. These results are valuable for improving our understanding of the sources and sinks of COS, contributing to the use of COS as a tracer for GPP.

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    Biogeosciences (BG)
    Other literature type . 2023
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    Research@WUR
    Other literature type . 2023
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    Biogeosciences
    Article . 2023 . Peer-reviewed
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    DOAJ
    Article . 2023
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      Research@WUR
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      Biogeosciences
      Article . 2023 . Peer-reviewed
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      Article . 2023
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    Authors: Fange Yue; Hélène Angot; Byron Blomquist; Julia Schmale; +20 Authors

    AbstractAtmospheric gaseous elemental mercury (GEM) concentrations in the Arctic exhibit a clear summertime maximum, while the origin of this peak is still a matter of debate in the community. Based on summertime observations during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition and a modeling approach, we further investigate the sources of atmospheric Hg in the central Arctic. Simulations with a generalized additive model (GAM) show that long-range transport of anthropogenic and terrestrial Hg from lower latitudes is a minor contribution (~2%), and more than 50% of the explained GEM variability is caused by oceanic evasion. A potential source contribution function (PSCF) analysis further shows that oceanic evasion is not significant throughout the ice-covered central Arctic Ocean but mainly occurs in the Marginal Ice Zone (MIZ) due to the specific environmental conditions in that region. Our results suggest that this regional process could be the leading contributor to the observed summertime GEM maximum. In the context of rapid Arctic warming and the observed increase in width of the MIZ, oceanic Hg evasion may become more significant and strengthen the role of the central Arctic Ocean as a summertime source of atmospheric Hg.

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    Nature Communications
    Article . 2023 . Peer-reviewed
    License: CC BY
    Data sources: Crossref
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      Nature Communications
      Article . 2023 . Peer-reviewed
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    Authors: I. Urzainki; I. Urzainki; M. Palviainen; H. Hökkä; +7 Authors

    Drainage in tropical peatlands increases CO2 emissions, the rate of subsidence, and the risk of forest fires. To a certain extent, these effects can be mitigated by raising the water table depth (WTD) using canal or ditch blocks. The performance of canal blocks in raising WTD is, however, poorly understood because the WTD monitoring data are limited and spatially concentrated around canals and canal blocks. This raises the following question: how effective are canal blocks in raising the WTD over large areas? In this work, we composed a process-based hydrological model to assess the peatland restoration performance of 168 canal blocks in a 22 000 ha peatland area in Sumatra, Indonesia. We simulated daily WTD over 1 year using an existing canal block setup and compared it to the situation without blocks. The study was performed across two contrasting weather scenarios representing dry (1997) and wet (2013) years. Our simulations revealed that, while canal blocks had a net positive impact on WTD rise, they lowered WTD in some areas, and the extent of their effect over 1 year was limited to a distance of about 600 m around the canals. We also show that canal blocks are most effective in peatlands with high hydraulic conductivity. Averaging over all modeled scenarios, blocks raised the annual mean WTD by only 1.5 cm. This value was similar in the dry (1.44 cm) and wet (1.57 cm) years, and there was a 2.13 fold difference between the scenarios with large and small hydraulic conductivities (2.05 cm versus 0.96 cm). Using a linear relationship between WTD and CO2 emissions, we estimated that, averaging over peat hydraulic properties, canal blocks prevented the emission of 1.07 Mg ha−1 CO2 in the dry year and 1.17 Mg ha−1 CO2 in the wet year. We believe that the modeling tools developed in this work could be adopted by local stakeholders aiming at a more effective and evidence-based approach to canal-block-based peatland restoration.

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    Biogeosciences
    Article . 2023 . Peer-reviewed
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    Biogeosciences (BG)
    Other literature type . 2023
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      Biogeosciences
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    Authors: Nie, Wei; Yan, Chao; Yang, Liwen; Roldin, Pontus; +48 Authors

    AbstractThe interaction between nitrogen monoxide (NO) and organic peroxy radicals (RO2) greatly impacts the formation of highly oxygenated organic molecules (HOM), the key precursors of secondary organic aerosols. It has been thought that HOM production can be significantly suppressed by NO even at low concentrations. Here, we perform dedicated experiments focusing on HOM formation from monoterpenes at low NO concentrations (0 – 82 pptv). We demonstrate that such low NO can enhance HOM production by modulating the RO2loss and favoring the formation of alkoxy radicals that can continue to autoxidize through isomerization. These insights suggest that HOM yields from typical boreal forest emissions can vary between 2.5%-6.5%, and HOM formation will not be completely inhibited even at high NO concentrations. Our findings challenge the notion that NO monotonically reduces HOM yields by extending the knowledge of RO2-NO interactions to the low-NO regime. This represents a major advance towards an accurate assessment of HOM budgets, especially in low-NO environments, which prevails in the pre-industrial atmosphere, pristine areas, and the upper boundary layer.

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    NRC Publications Archive; Nature Communications
    Other literature type . Article . 2023 . Peer-reviewed
    License: CC BY
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    CERN Document Server
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      NRC Publications Archive; Nature Communications
      Other literature type . Article . 2023 . Peer-reviewed
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Victoria Reyes-García; David García-del-Amo; Santiago Álvarez-Fernández; Petra Benyei; +54 Authors

    AbstractThe effects of climate change depend on specific local circumstances, posing a challenge for worldwide research to comprehensively encompass the diverse impacts on various local social-ecological systems. Here we use a place-specific but cross-culturally comparable protocol to document climate change indicators and impacts as locally experienced and analyze their distribution. We collected first-hand data in 48 sites inhabited by Indigenous Peoples and local communities and covering all climate zones and nature-dependent livelihoods. We documented 1,661 site-agreed reports of change corresponding to 369 indicators. Reports of change vary according to climate zone and livelihood activity. We provide compelling evidence that climate change impacts on Indigenous Peoples and local communities are ongoing, tangible, widespread, and affect multiple elements of their social-ecological systems. Beyond potentially informing contextualized adaptation plans, our results show that local reports could help identify economic and non-economic loss and damage related to climate change impacts suffered by Indigenous Peoples and local communities.

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    Research@WUR; Communications Earth & Environment
    Other literature type . Article . 2024 . Peer-reviewed
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      Research@WUR; Communications Earth & Environment
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    Authors: Xiansheng, Liu; Hadiatullah, Hadiatullah; Xun, Zhang; Pedro, Trechera; +48 Authors

    This study is supported by the RI-URBANS project (Research Infrastructures Services Reinforcing Air Quality Monitoring Capacities in European Urban & amp; Industrial Areas, European Union's Horizon 2020 research and innovation program, Green Deal, European Commission, contract 101036245). This study is also supported by National Natural Science Foundation of China (42101470, 72242106) and in part by the Chunhui Project Foundation of the Education Department of China under Grant HZKY20220053. This study benefited from the Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS), especially the so-called ACTRIS-2 H2020 research project (grant no 654109), and the authors would like to thank ACTRIS (The Aerosol, Clouds and Trace Gases Research Infrastructure), especially the ACTRIS in situ EBAS Data Centre (EBAS), for providing datasets to the study. This study is also partly funded by the National Institute for Health Research (NIHR) Health Protection Research Unit in Environmental Exposures and Health, a partnership between UK Health Security Agency (UKHSA) and Imperial College London, and the UK Natural Environment Re-search Council, and the views expressed are those of the author(s) and not necessarily those of the NIHR, UKHSA or the Department of Health and Social Care. The research was also supported by the Hungarian Research, Development and Innovation Office (grant no. K132254). We thank also the support from "Agencia Estatal de Investigacion" from the Spanish Ministry of Science and Innovation, and FEDER funds under the projects CAIAC (PID2019-108990RB-I00); and the Generalitat de Catalunya (AGAUR 2017 SGR41) and the Direccio General de Territori. IMT Nord Europe and LOA acknowledge financial support from the Labex CaPPA project, funded by the French National Research Agency (ANR-11-LABX-0005-01), and the CLIMIBIO and ECRIN projects, both financed by the Regional Council "Hauts-de-France" and the European Regional Development Fund (ERDF). This study aims to picture the phenomenology of urban ambient total lung deposited surface area (LDSA) (including head/throat (HA), tracheobronchial (TB), and alveolar (ALV) regions) based on multiple path particle dosimetry (MPPD) model during 2017-2019 period collected from urban background (UB, n = 15), traffic (TR, n = 6), suburban background (SUB, n = 4), and regional background (RB, n = 1) monitoring sites in Europe (25) and USA (1). Briefly, the spatial-temporal distribution characteristics of the deposition of LDSA, including diel, weekly, and seasonal pat-terns, were analyzed. Then, the relationship between LDSA and other air quality metrics at each monitoring site was investigated. The result showed that the peak concentrations of LDSA at UB and TR sites are commonly observed in the morning (06:00-8:00 UTC) and late evening (19:00-22:00 UTC), coinciding with traffic rush hours, biomass burning, and atmospheric stagnation periods. The only LDSA night-time peaks are observed on weekends. Due to the variability of emission sources and meteorology, the seasonal variability of the LDSA concentration revealed sig-nificant differences (p = 0.01) between the four seasons at all monitoring sites. Meanwhile, the correlations of LDSA with other pollutant metrics suggested that Aitken and accumulation mode particles play a significant role in the total LDSA concentration. The results also indicated that the main proportion of total LDSA is attributed to the ALV fraction (50 %), followed by the TB (34 %) and HA (16 %). Overall, this study provides valuable information of LDSA as a predictor in epidemiological studies and for the first time presenting total LDSA in a variety of European urban environments. RI-URBANS project (Research Infrastructures Services Reinforcing Air Quality Monitoring Capacities in European Urban amp; Industrial Areas, European Union's Horizon 2020 research and innovation program, Green Deal, European Commission, 101036245) National Institute for Health Research (NIHR) Health Protection Research Unit in Environmental Exposures and Health European Union (EU) K132254, PID2019-108990RB-I00, AGAUR 2017 SGR41, ANR-11-LABX-0005-01 "Agencia Estatal de Investigacion" from the Spanish Ministry of Science and Innovation UK Research & Innovation (UKRI) Natural Environment Research Council (NERC) National Research, Development & Innovation Office (NRDIO) - Hungary Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS) Chunhui Project Foundation of the Education Department of China National Natural Science Foundation of China (NSFC) Agence Nationale de la Recherche (ANR) 654109 Generalitat de Catalunya 42101470, 72242106 Direccio General de Territori HZKY20220053 Regional Council "Hauts-de-France" ERDF

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    Lille Open Archive
    Article . 2023
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    Authors: M. J. Campmier; J. Gingrich; S. Singh; N. Baig; +12 Authors

    Lower-cost air pollution sensors can fill critical air quality data gaps in India, which experiences very high fine particulate matter (PM2.5) air pollution but has sparse regulatory air monitoring. Challenges for low-cost PM2.5 sensors in India include high-aerosol mass concentrations and pronounced regional and seasonal gradients in aerosol composition. Here, we report on a detailed long-time performance evaluation of a popular sensor, the Purple Air PA-II, at multiple sites in India. We established three distinct sites in India across land use categories and population density extremes (in urban Delhi and rural Hamirpur in north India and urban Bengaluru in south India), where we collocated the PA-II model with reference beta attenuation monitors. We evaluated the performance of uncalibrated sensor data, and then developed, optimized, and evaluated calibration models using a comprehensive feature selection process with a view to reproducibility in the Indian context. We assessed the seasonal and spatial transferability of sensor calibration schemes, which is especially important in India because of the paucity of reference instrumentation. Without calibration, the PA-II was moderately correlated with the reference signal (R2 = 0.55–0.74) but was inaccurate (NRMSE ≥ 40 %). Relative to uncalibrated data, parsimonious annual calibration models improved the PurpleAir (PA) model performance at all sites (cross-validated NRMSE 20 %–30 %; R2 = 0.82–0.95), and greatly reduced seasonal and diurnal biases. Because aerosol properties and meteorology vary regionally, the form of these long-term models differed among our sites, suggesting that local calibrations are desirable when possible. Using a moving-window calibration, we found that using seasonally specific information improves performance relative to a static annual calibration model, while a short-term calibration model generally does not transfer reliably to other seasons. Overall, we find that the PA-II model can provide reliable PM2.5 data with better than ±25 % precision and accuracy when paired with a rigorous calibration scheme that accounts for seasonality and local aerosol composition.

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    Atmospheric Measurement Techniques
    Article . 2023 . Peer-reviewed
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      Atmospheric Measurement Techniques
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    Authors: M. J. McGrath; A. M. R. Petrescu; P. Peylin; R. M. Andrew; +69 Authors

    Quantification of land surface–atmosphere fluxes of carbon dioxide (CO2) and their trends and uncertainties is essential for monitoring progress of the EU27+UK bloc as it strives to meet ambitious targets determined by both international agreements and internal regulation. This study provides a consolidated synthesis of fossil sources (CO2 fossil) and natural (including formally managed ecosystems) sources and sinks over land (CO2 land) using bottom-up (BU) and top-down (TD) approaches for the European Union and United Kingdom (EU27+UK), updating earlier syntheses (Petrescu et al., 2020, 2021). Given the wide scope of the work and the variety of approaches involved, this study aims to answer essential questions identified in the previous syntheses and understand the differences between datasets, particularly for poorly characterized fluxes from managed and unmanaged ecosystems. The work integrates updated emission inventory data, process-based model results, data-driven categorical model results, and inverse modeling estimates, extending the previous period 1990–2018 to the year 2020 to the extent possible. BU and TD products are compared with the European national greenhouse gas inventory (NGHGI) reported by parties including the year 2019 under the United Nations Framework Convention on Climate Change (UNFCCC). The uncertainties of the EU27+UK NGHGI were evaluated using the standard deviation reported by the EU member states following the guidelines of the Intergovernmental Panel on Climate Change (IPCC) and harmonized by gap-filling procedures. Variation in estimates produced with other methods, such as atmospheric inversion models (TD) or spatially disaggregated inventory datasets (BU), originate from within-model uncertainty related to parameterization as well as structural differences between models. By comparing the NGHGI with other approaches, key sources of differences between estimates arise primarily in activities. System boundaries and emission categories create differences in CO2 fossil datasets, while different land use definitions for reporting emissions from land use, land use change, and forestry (LULUCF) activities result in differences for CO2 land. The latter has important consequences for atmospheric inversions, leading to inversions reporting stronger sinks in vegetation and soils than are reported by the NGHGI. For CO2 fossil emissions, after harmonizing estimates based on common activities and selecting the most recent year available for all datasets, the UNFCCC NGHGI for the EU27+UK accounts for 926 ± 13 Tg C yr−1, while eight other BU sources report a mean value of 948 [937,961] Tg C yr−1 (25th, 75th percentiles). The sole top-down inversion of fossil emissions currently available accounts for 875 Tg C in this same year, a value outside the uncertainty of both the NGHGI and bottom-up ensemble estimates and for which uncertainty estimates are not currently available. For the net CO2 land fluxes, during the most recent 5-year period including the NGHGI estimates, the NGHGI accounted for −91 ± 32 Tg C yr−1, while six other BU approaches reported a mean sink of −62 [-117,-49] Tg C yr−1, and a 15-member ensemble of dynamic global vegetation models (DGVMs) reported −69 [-152,-5] Tg C yr−1. The 5-year mean of three TD regional ensembles combined with one non-ensemble inversion of −73 Tg C yr−1 has a slightly smaller spread (0th–100th percentiles of [-135,+45] Tg C yr−1), and it was calculated after removing net land–atmosphere CO2 fluxes caused by lateral transport of carbon (crop trade, wood trade, river transport, and net uptake from inland water bodies), resulting in increased agreement with the NGHGI and bottom-up approaches. Results at the category level (Forest Land, Cropland, Grassland) generally show good agreement between the NGHGI and category-specific models, but results for DGVMs are mixed. Overall, for both CO2 fossil and net CO2 land fluxes, we find that current independent approaches are consistent with the NGHGI at the scale of the EU27+UK. We conclude that CO2 emissions from fossil sources have decreased over the past 30 years in the EU27+UK, while land fluxes are relatively stable: positive or negative trends larger (smaller) than 0.07 (−0.61) Tg C yr−2 can be ruled out for the NGHGI. In addition, a gap on the order of 1000 Tg C yr−1 between CO2 fossil emissions and net CO2 uptake by the land exists regardless of the type of approach (NGHGI, TD, BU), falling well outside all available estimates of uncertainties. However, uncertainties in top-down approaches to estimate CO2 fossil emissions remain uncharacterized and are likely substantial, in addition to known uncertainties in top-down estimates of the land fluxes. The data used to plot the figures are available at https://doi.org/10.5281/zenodo.8148461 (McGrath et al., 2023).

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    MPG.PuRe
    Article . 2023
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    Earth System Science Data (ESSD)
    Other literature type . 2023
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    Article . 2023
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      MPG.PuRe
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    Authors: M. Räsänen; R. Vesala; P. Rönnholm; L. Arppe; +8 Authors

    Termites play an essential role in decomposing dead plant material in tropical ecosystems and are thus major sources of gaseous C emissions in many environments. In African savannas, fungus-growing termites are among the ecologically most influential termite species. We studied the gas exchange from mounds of two closely related fungus-growing species (Macrotermes subhyalinus and M. michaelseni, respectively) in two habitats representing different vegetation types (grassland, bushland) together with soil fluxes around the mounds. The fluxes from active termite mounds varied from 120 to 2100 mg CO2–C m−2 h−1 for carbon dioxide (CO2) and from 0.06 to 3.7 mg CH4–C m−2 h−1 for methane (CH4) fluxes. Mound CO2 fluxes varied seasonally with a 64 % decrease and 41 % increase in the fluxes from the dry to wet season at the grassland and bushland sites, respectively. During the wet season, the CO2 fluxes were significantly correlated with termite mound volume. The diurnal measurements from two M. michaelseni mounds suggest that the gas fluxes peak during the daytime, possibly reflecting changes in mound internal air circulation. Soil fluxes of both CO2 and CH4 were enhanced at up to 2 m distance from the mounds compared to the local soil respiration, indicating that, in addition to mound ventilation structures, a small proportion of the metabolic gases produced also leave the nest via surrounding soils.

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    Biogeosciences (BG)
    Other literature type . 2023
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    Aaltodoc Publication Archive
    Article . 2023 . Peer-reviewed
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    Biogeosciences
    Article . 2023 . Peer-reviewed
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    DOAJ
    Article . 2023
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      Biogeosciences (BG)
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      Aaltodoc Publication Archive
      Article . 2023 . Peer-reviewed
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      Biogeosciences
      Article . 2023 . Peer-reviewed
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      Article . 2023
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    Authors: Lubna Dada; Dominik Stolzenburg; Mario Simon; Lukas Fischer; +51 Authors

    Biogenic vapors form new particles in the atmosphere, affecting global climate. The contributions of monoterpenes and isoprene to new particle formation (NPF) have been extensively studied. However, sesquiterpenes have received little attention despite a potentially important role due to their high molecular weight. Via chamber experiments performed under atmospheric conditions, we report biogenic NPF resulting from the oxidation of pure mixtures of beta-caryophyllene, alpha-pinene, and isoprene, which produces oxygenated compounds over a wide range of volatilities. We find that a class of vapors termed ultralow-volatility organic compounds (ULVOCs) are highly efficient nucleators and quantitatively determine NPF efficiency. When compared with a mixture of isoprene and monoterpene alone, adding only 2% sesquiterpene increases the ULVOC yield and doubles the formation rate. Thus, sesquiterpene emissions need to be included in assessments of global aerosol concentrations in pristine climates where biogenic NPF is expected to be a major source of cloud condensation nuclei. Peer reviewed

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    Science Advances
    Article . 2023 . Peer-reviewed
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    KITopen
    Article . 2023
    License: CC BY NC
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    https://doi.org/10.5445/ir/100...
    Article . 2023
    License: CC BY NC
    Data sources: Datacite
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    CERN Document Server
    Other literature type . 2023
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    Science Advances
    Article . 2023
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      Science Advances
      Article . 2023 . Peer-reviewed
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      KITopen
      Article . 2023
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      https://doi.org/10.5445/ir/100...
      Article . 2023
      License: CC BY NC
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      CERN Document Server
      Other literature type . 2023
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      Science Advances
      Article . 2023
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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    Authors: A. Zanchetta; L. M. J. Kooijmans; L. M. J. Kooijmans; S. van Heuven; +9 Authors

    Carbonyl sulfide (COS) is a promising tracer for the estimation of terrestrial ecosystem gross primary production (GPP). However, understanding its non-GPP-related sources and sinks, e.g., anthropogenic sources and soil sources and sinks, is also critical to the success of the approach. Here we infer the regional sources and sinks of COS using continuous in situ mole fraction profile measurements of COS along the 60 m tall Lutjewad tower (1 m a.s.l.; 53∘24′ N, 6∘21′ E) in the Netherlands. To identify potential sources that caused the observed enhancements of COS mole fractions at Lutjewad, both discrete flask samples and in situ measurements in the province of Groningen were made from a mobile van using a quantum cascade laser spectrometer (QCLS). We also simulated the COS mole fractions at Lutjewad using the Stochastic Time-Inverted Lagrangian Transport (STILT) model combined with emission inventories and plant uptake fluxes. We determined the nighttime COS fluxes to be -3.0±2.6 pmol m−2 s−1 using the radon-tracer correlation approach and Lutjewad observations. Furthermore, we identified and quantified several COS sources, including biodigesters, sugar production facilities and silicon carbide production facilities in the province of Groningen. Moreover, the simulation results show that the observed COS enhancements can be partially explained by known industrial sources of COS and CS2, in particular from the Ruhr Valley (51.5∘ N, 7.2∘ E) and Antwerp (51.2∘ N, 4.4∘ E) areas. The contribution of likely missing anthropogenic sources of COS and CS2 in the inventory may be significant. The impact of the identified sources in the province of Groningen is estimated to be negligible in terms of the observed COS enhancements. However, in specific conditions, these sources may influence the measurements in Lutjewad. These results are valuable for improving our understanding of the sources and sinks of COS, contributing to the use of COS as a tracer for GPP.

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    Biogeosciences (BG)
    Other literature type . 2023
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    Research@WUR
    Other literature type . 2023
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    Biogeosciences
    Article . 2023 . Peer-reviewed
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    DOAJ
    Article . 2023
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      Biogeosciences (BG)
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      Research@WUR
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      Biogeosciences
      Article . 2023 . Peer-reviewed
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      Article . 2023
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    Authors: Fange Yue; Hélène Angot; Byron Blomquist; Julia Schmale; +20 Authors

    AbstractAtmospheric gaseous elemental mercury (GEM) concentrations in the Arctic exhibit a clear summertime maximum, while the origin of this peak is still a matter of debate in the community. Based on summertime observations during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition and a modeling approach, we further investigate the sources of atmospheric Hg in the central Arctic. Simulations with a generalized additive model (GAM) show that long-range transport of anthropogenic and terrestrial Hg from lower latitudes is a minor contribution (~2%), and more than 50% of the explained GEM variability is caused by oceanic evasion. A potential source contribution function (PSCF) analysis further shows that oceanic evasion is not significant throughout the ice-covered central Arctic Ocean but mainly occurs in the Marginal Ice Zone (MIZ) due to the specific environmental conditions in that region. Our results suggest that this regional process could be the leading contributor to the observed summertime GEM maximum. In the context of rapid Arctic warming and the observed increase in width of the MIZ, oceanic Hg evasion may become more significant and strengthen the role of the central Arctic Ocean as a summertime source of atmospheric Hg.

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    Nature Communications
    Article . 2023 . Peer-reviewed
    License: CC BY
    Data sources: Crossref
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    DOAJ
    Article . 2023
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      Nature Communications
      Article . 2023 . Peer-reviewed
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      Article . 2023
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    Authors: I. Urzainki; I. Urzainki; M. Palviainen; H. Hökkä; +7 Authors

    Drainage in tropical peatlands increases CO2 emissions, the rate of subsidence, and the risk of forest fires. To a certain extent, these effects can be mitigated by raising the water table depth (WTD) using canal or ditch blocks. The performance of canal blocks in raising WTD is, however, poorly understood because the WTD monitoring data are limited and spatially concentrated around canals and canal blocks. This raises the following question: how effective are canal blocks in raising the WTD over large areas? In this work, we composed a process-based hydrological model to assess the peatland restoration performance of 168 canal blocks in a 22 000 ha peatland area in Sumatra, Indonesia. We simulated daily WTD over 1 year using an existing canal block setup and compared it to the situation without blocks. The study was performed across two contrasting weather scenarios representing dry (1997) and wet (2013) years. Our simulations revealed that, while canal blocks had a net positive impact on WTD rise, they lowered WTD in some areas, and the extent of their effect over 1 year was limited to a distance of about 600 m around the canals. We also show that canal blocks are most effective in peatlands with high hydraulic conductivity. Averaging over all modeled scenarios, blocks raised the annual mean WTD by only 1.5 cm. This value was similar in the dry (1.44 cm) and wet (1.57 cm) years, and there was a 2.13 fold difference between the scenarios with large and small hydraulic conductivities (2.05 cm versus 0.96 cm). Using a linear relationship between WTD and CO2 emissions, we estimated that, averaging over peat hydraulic properties, canal blocks prevented the emission of 1.07 Mg ha−1 CO2 in the dry year and 1.17 Mg ha−1 CO2 in the wet year. We believe that the modeling tools developed in this work could be adopted by local stakeholders aiming at a more effective and evidence-based approach to canal-block-based peatland restoration.

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    Biogeosciences
    Article . 2023 . Peer-reviewed
    License: CC BY
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    Biogeosciences (BG)
    Other literature type . 2023
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    DOAJ
    Article . 2023
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      Biogeosciences
      Article . 2023 . Peer-reviewed
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    Authors: Nie, Wei; Yan, Chao; Yang, Liwen; Roldin, Pontus; +48 Authors

    AbstractThe interaction between nitrogen monoxide (NO) and organic peroxy radicals (RO2) greatly impacts the formation of highly oxygenated organic molecules (HOM), the key precursors of secondary organic aerosols. It has been thought that HOM production can be significantly suppressed by NO even at low concentrations. Here, we perform dedicated experiments focusing on HOM formation from monoterpenes at low NO concentrations (0 – 82 pptv). We demonstrate that such low NO can enhance HOM production by modulating the RO2loss and favoring the formation of alkoxy radicals that can continue to autoxidize through isomerization. These insights suggest that HOM yields from typical boreal forest emissions can vary between 2.5%-6.5%, and HOM formation will not be completely inhibited even at high NO concentrations. Our findings challenge the notion that NO monotonically reduces HOM yields by extending the knowledge of RO2-NO interactions to the low-NO regime. This represents a major advance towards an accurate assessment of HOM budgets, especially in low-NO environments, which prevails in the pre-industrial atmosphere, pristine areas, and the upper boundary layer.

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    NRC Publications Archive; Nature Communications
    Other literature type . Article . 2023 . Peer-reviewed
    License: CC BY
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    CERN Document Server
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    DOAJ
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      NRC Publications Archive; Nature Communications
      Other literature type . Article . 2023 . Peer-reviewed
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